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Part I: Basic Properties and Early Works in Organic–Inorganic Perovskites
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Part I: Basic Properties and Early Works in Organic–Inorganic Perovskites
by Nripan Mathews, Tze-Chien Sum
Halide Perovskites
Cover
Dedication
Part I: Basic Properties and Early Works in Organic–Inorganic Perovskites
1.1 Structural, Optical, and Related Properties of Some Perovskites Based on Lead and Tin Halides: The Effects on Going from Bulk to Small Particles
1.1.1 Introduction
1.1.2 Materials Based on Saturated Organic Moiety
1.1.3 Perovskites Consisting of Non‐saturated Organic Moiety BC
1.1.4 Other Perovskite Structures
References
1.2 Ab Initio and First Principles Studies of Halide Perovskites
1.2.1 Introduction to Ab Initio and DFT Studies of All‐inorganic, 3D and Layered Hybrid Organic Metal Halide Perovskites
1.2.2 Brillouin Zone Folding, Lattice Strain, and Topology of the Electronic Structure
1.2.3 Importance of Spin–Orbit Coupling (SOC)
1.2.4 Interplay of SOC and Loss of Inversion Symmetry: Rashba and Dresselhaus Effects
1.2.5 Collective Vibrations, Stochastic Cation Reorientations, and Molecular Dynamics
References
1.3 Excitonics in 2D Perovskites
1.3.1 Introduction to Two‐dimensional Perovskites
1.3.2 Excitonic Properties and Optical Transitions in 2D‐OIHPs
1.3.3 White Light Emission (WLE) from 2D‐OIHPs
1.3.4 Strong Exciton–Photon Coupling in 2D‐OIHPs
1.3.5 Concluding Remarks
References
Part II: Organic–Inorganic Perovskite Solar Cells
2.1 Working Principles of Perovskite Solar Cells
2.1.1 Introduction
2.1.2 Charge Generation
2.1.3 Charge Transport
2.1.4 Charge Recombination
2.1.5 Charge Extraction/Injection: Interfacial Effects
2.1.6 Ionic Mechanisms
2.1.7 Concluding Remarks
References
2.2 The Photophysics of Halide Perovskite Solar Cells
2.2.1 Introduction to Photophysics Studies of Halide Perovskites
2.2.2 Optical Properties of CH3NH3PbI3 Polycrystalline Thin Films
2.2.3 Energetics and Charge Dynamics at Perovskite Interfaces
2.2.4 Toward Perovskite Single‐Crystal Photovoltaics
2.2.5 Concluding Remarks
References
2.3 Charge‐Selective Contact Materials for Perovskite Solar Cells (PSCs)
2.3.1 Hole‐Selective Electron‐Blocking Materials (HTMs)
2.3.2 Electron‐Selective Hole‐Blocking Materials
2.3.3 Conclusion
References
2.4 Beyond Methylammonium Lead Iodide Perovskite
2.4.1 Introduction: Beyond CH3NH3PbI3
2.4.2 Theoretical Calculations for Pb‐Free Halide Perovskites
2.4.3 Experimental Efforts in Pb‐Free Perovskite Photovoltaics
2.4.4 Concluding Remarks and Outlook
References
2.5 Halide Perovskite Tandem Solar Cells
2.5.1 Introduction
2.5.2 Tandem Device Type and Performance Limitations
2.5.3 Perovskite Tandem Photovoltaic Device Research
2.5.4 Conclusion and Outlook
References
Part III: Perovskite Light Emitting Devices
3.1 Perovskite Light‐Emitting Devices – Fundamentals and Working Principles
3.1.1 Excitons, Free Carriers, and Trap States in Hybrid Perovskite Thin Films
3.1.2 Hybrid Perovskite Light‐Emitting Diodes
3.1.3 Hybrid Perovskite Nanostructures and Nanoparticles
References
3.2 Toward Electrically Driven Perovskite Lasers – Prospects and Obstacles
3.2.1 Introduction
3.2.2 Electrical Injection in Perovskite‐Based Light‐Emitting Diodes (LEDs)
3.2.3 Optical Gain in Thin‐film Solid‐state Perovskites
3.2.4 Integrating Optical Resonators and Perovskite Gain Media
3.2.5 The Way Forward Toward Electrical Injection
3.2.6 Summary
References
Part IV: Beyond Perovskite Photovoltaics
4.1 Novel Spin Physics in Organic–Inorganic Perovskites
4.1.1 Introduction
4.1.2 Magnetic Field Effect (MFE) on Photocurrent (PC), Photoluminescence (PL), and Electroluminescence (EL)
4.1.3 High Magnetic Field Optical Phenomena
4.1.4 Spin‐Polarized Carrier Dynamics
4.1.5 Conclusion and Outlook
Acknowledgements
References
4.2 Perovskite Solar Cells for Photoelectrochemical Water Splitting and CO2 Reduction
4.2.1 Introduction
4.2.2 Tandem Configurations
4.2.3 EC/PEC‐PV Approach for CO2 Reduction
4.2.4 Concluding Remarks and Outlook
References
Index
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1.1 Structural, Optical, and Related Properties of Some Perovskites Based on Lead and Tin Halides: The Effects on Going from Bulk to Small Particles
Part I
Basic Properties and Early Works in Organic–Inorganic Perovskites
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